A spherically expanding flame in a quiescent premixture is a bifurcation phenomenon, in which the flame becomes unstable at a radius, greater than some critical value, while remaining stable below that critical radius. Beyond this critical radius, developing instabilities are initiated by propagating cracks to form a coherent structure covering the entire flame surface and the flame accelerates. The present paper reports a Schlieren photographic study of spherical flame propagation in methane—air, iso-octane—air and n-heptane—air premixtures at different initial conditions where the onset of instability and the flame acceleration are clearly perceived. Critical size and corresponding elapsed time for the development of such instability are measured and these values are correlated with the appropriate flame parameter.

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